Aldehydes and ketones: properties, reactions, tests

Aldehydes and Ketones (Cambridge AS/A‑Level – Topic 18)

Learning outcomes (syllabus mapping)

  • Identify and name aldehydes and ketones (IUPAC, common names, skeletal formulas).
  • Explain the electronic structure of the carbonyl group (resonance, polarity, partial charges).
  • Predict physical properties (polarity, solubility, boiling‑point trends) from structure.
  • Describe the general reactivity of carbonyl compounds – nucleophilic addition, oxidation, reduction, and protection.
  • Write mechanisms for the key reactions: nucleophilic addition, Grignard addition, acetal formation, enolate chemistry, aldol condensation, Wittig olefination.
  • Carry out and interpret the classical qualitative tests (Fehling, Tollens, Schiff, 2,4‑DNP, Jones).
  • Use oxidation‑state concepts to rationalise oxidation and oxidative cleavage.
  • Apply practical exam tips for quick, accurate answers.

1. Naming & basic formulas

Common name IUPAC name Structural formula Skeletal formula
Formaldehyde Methanal H‑C(=O)‑H H‑C=O
Acetaldehyde Ethanal CH₃‑C(=O)‑H CH₃‑C=O
Acetone Propan‑2‑one CH₃‑C(=O)‑CH₃ CH₃‑C=O‑CH₃
Cyclohexanone Cyclohexan‑one C₆H₁₀‑C(=O)‑ ⟳‑C=O

2. Electronic structure of the carbonyl group

  • Dominant resonance form: R‑C(=O)‑R′ ⇌ R‑C⁺‑O⁻‑R′
  • Resulting partial charges: δ⁺ on carbonyl carbon (≈ +0.5 – +1.0 e) and δ⁻ on oxygen (≈ ‑0.5 e).
  • Consequences:
    • Carbonyl carbon is electrophilic → susceptible to nucleophilic attack.
    • In aldehydes the carbonyl carbon is less hindered, giving a larger δ⁺ and higher reactivity than in ketones.

3. Physical properties

Property Aldehyde (R‑CHO) Ketone (R‑CO‑R′)
Polarity Carbonyl C=O is strongly polar; the –CHO hydrogen can act as a H‑bond donor as well as the oxygen as an acceptor. Carbonyl C=O is polar; no H‑bond donor – only H‑bond acceptance.
Solubility in water ≤ C₄ aldehydes (formaldehyde, acetaldehyde, propionaldehyde) are miscible; solubility falls with chain length. Generally less soluble than comparable aldehydes because of the missing H‑bond donor.
Boiling‑point trend
  • ≈ 5 °C (≈ 2 kJ mol⁻¹) rise per added –CH₂–.
  • Lower than ketones of the same molecular weight: less steric bulk → weaker dipole‑dipole interactions; very small aldehydes benefit from H‑bond donation.
  • ≈ 5 °C increase per –CH₂–.
  • Higher than aldehydes of the same formula because two alkyl groups increase the dipole moment and steric hindrance.
Reactivity toward nucleophiles More electrophilic (δ⁺ ≈ +1); carbonyl carbon is less hindered. Less electrophilic (δ⁺ ≈ +0.5) but still undergoes addition.

4. General reactivity overview

  • Nucleophilic addition – the principal reaction mode for both families.
  • Oxidation – aldehydes → carboxylic acids (mild oxidants). Ketones require strong oxidisers for C–C cleavage.
  • Reduction – both are reduced to alcohols; aldehydes give primary, ketones give secondary alcohols.
  • Acid‑catalysed hydration – reversible formation of gem‑diols (hydrates), illustrating the addition mechanism.
  • Protection – conversion to acetals or ketals under acidic conditions.

5. Key mechanisms

5.1. General nucleophilic addition

R‑C(=O)‑R′  +  Nu⁻   →   R‑C(–O⁻)(‑Nu)‑R′   (tetrahedral alkoxide)
R‑C(–O⁻)(‑Nu)‑R′   +   H⁺   →   R‑C(=O‑H)(‑Nu)‑R′
  • Curly‑arrow steps:
    1. Nu⁻ donates a lone pair to the carbonyl carbon.
    2. The π‑bond electrons move onto oxygen, giving O⁻.
    3. O⁻ is protonated by solvent or added acid.

5.2. Reduction

  • NaBH₄ (mild) – selective for aldehydes & ketones.
        R‑CHO   +   NaBH₄   →   R‑CH₂OH
        R‑CO‑R′ +   NaBH₄   →   R‑CH(OH)‑R′
        
  • LiAlH₄ (strong) – reduces aldehydes, ketones, esters, acids, acid chlorides, etc.

5.3. Grignard addition

R″MgX  +  R‑C(=O)‑R′   →   R‑C(–OMgX)(‑R″)‑R′   →   (H⁺)   R‑C(OH)(‑R″)‑R′
  • From aldehydes → secondary alcohols; from ketones → tertiary alcohols.

5.4. Acetal (ketal) formation – protection of carbonyls

R‑C(=O)‑R′  +  2 R″OH   ⇌   R‑C(OR″)₂‑R′  +  H₂O   (acid catalyst)
  • Acetals are stable to bases and nucleophiles; they are removed by aqueous acid.

5.5. Acid‑catalysed hydration (gem‑diol)

R‑CHO   +   H₂O   ⇌   R‑CH(OH)₂
R‑CO‑R′ +   H₂O   ⇌   R‑C(OH)₂‑R′
  • Equilibrium lies left for most carbonyls; electron‑withdrawing substituents (Cl, CN) shift it right.

5.6. Enolisation & enolate chemistry

R‑CH₂‑C(=O)‑R′   +   B⁻   →   R‑CH⁻‑C(=O)‑R′   (enolate)   +   HB
  • Base removes an α‑hydrogen, generating an enolate (nucleophilic at carbon).
  • Enol (R‑CH=​C(OH)‑R′) is the protonated tautomer; resonance between enolate and enol stabilises the intermediate.

5.7. Aldol condensation (base‑catalysed)

Enolate + R″‑CHO   →   β‑hydroxy carbonyl (aldol)
β‑hydroxy carbonyl   →(Δ)   α,β‑unsaturated carbonyl + H₂O
  • Requires at least one α‑hydrogen on the carbonyl that forms the enolate.
  • Typical exam example: acetone + benzaldehyde → benzalacetone (α,β‑unsaturated ketone).

5.8. Wittig olefination

Ph₃P=CH₂   +   R‑C(=O)‑R′   →   R‑CH=CH₂   +   Ph₃P=O
  • Phosphonium ylide attacks the carbonyl, forming a betaine that collapses to an alkene and triphenylphosphine oxide.
  • Choice of ylide (stabilised vs non‑stabilised) controls E/Z geometry.

6. Classical qualitative tests

Test Reagents / Conditions Observed result Interpretation
Fehling’s test Fehling A (CuSO₄) + Fehling B (KNaC₄H₄O₆), alkaline (NaOH) Brick‑red precipitate of Cu₂O Positive for aldehydes (including aromatic). No precipitate with ketones.
Tollens’ test AgNO₃ + NH₃ (ammoniacal Ag⁺), alkaline Silver mirror on glass (Ag⁰) Positive for aldehydes that possess an α‑hydrogen (most aliphatic aldehydes). α‑Keto‑aldehydes also give a positive test.
Schiff’s test Schiff’s reagent (de‑colourised fuchsin sulphurous acid) Pink to magenta colour Positive for aldehydes (including aromatic). Requires an α‑hydrogen for imine formation.
2,4‑DNP test 2,4‑Dinitrophenylhydrazine in acidic ethanol Yellow precipitate (aldehydes) or orange/red precipitate (ketones) Both give a hydrazone; colour helps distinguish the two.
Jones oxidation (chromic acid test) CrO₃ in aqueous H₂SO₄ (orange solution) Colour change orange → green (Cr³⁺) for aldehydes; no change for most ketones. Aldehyde is oxidised to the corresponding carboxylic acid; ketones are generally unchanged.

Why the α‑hydrogen matters: In Tollens, Schiff and aldol reactions the carbonyl must be able to form an imine or an enolate. The presence of an α‑hydrogen allows deprotonation → enolate → nucleophilic attack, giving a positive test or condensation product.

7. Oxidation‑state perspective & oxidative cleavage

Functional group Oxidation state of carbonyl carbon Typical oxidation Product(s)
Aldehyde (R‑CHO) +1 Fehling, Tollens, Jones (mild) Carboxylic acid (C = +3)
Ketone (R‑CO‑R′) +2 Strong oxidisers (KMnO₄, CrO₃) – oxidative C–C cleavage Two carboxylic acids (each C = +3)

Example: Oxidative cleavage of a symmetric ketone

R‑CO‑R   +   [O]   →   2 R‑COOH

8. Practical exam tips

  • Check for an α‑hydrogen first. Its presence tells you:
    • If the compound can undergo enolate chemistry (aldol, alkylation).
    • Whether Tollens or Schiff tests will be positive.
  • Boiling‑point comparisons
    • Count –CH₂– groups (≈ 5 °C per group).
    • Remember: very small aldehydes can H‑bond donate → slightly higher b.p. than expected.
    • Ketones are usually higher than aldehydes of the same molecular weight because of greater steric bulk around the carbonyl.
  • 2,4‑DNP colour cue
    • Yellow → aldehyde.
    • Orange/red → ketone.
  • Reduction questions
    • NaBH₄ = selective for aldehydes & ketones only.
    • LiAlH₄ = reduces a broader range (esters, acids, acid chlorides, etc.).
  • Protecting a carbonyl – write the acetal formation using a diol (e.g., ethylene glycol → cyclic acetal).
  • Jones oxidation colour change – orange (Cr(VI)) → green (Cr(III)) indicates oxidation of an aldehyde; ketones remain orange.
  • Mechanism drawing – in the exam booklet, sketch the nucleophilic addition curly‑arrow sequence (attack, alkoxide, protonation) for full credit.

9. Suggested diagrams for the exam booklet

  1. Resonance structures of the carbonyl group showing δ⁺ on carbon and δ⁻ on oxygen.
  2. Curly‑arrow mechanism of a generic nucleophilic addition (including protonation).
  3. Enolate formation from a carbonyl with an α‑hydrogen (base‑catalysed).
  4. Aldol condensation (enolate attack → β‑hydroxy carbonyl → dehydration).
  5. Acetal formation from a ketone and ethylene glycol (showing acid catalyst and water removal).

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